| Citation: | XIE Song, PING Xianke, GONG Yizeet al. Effect of high altitude and low pressure on cycle performance of lithium-ion batteries[J]. Journal of Beijing University of Aeronautics and Astronautics, 2022, 48(10): 1883-1888. doi: 10.13700/j.bh.1001-5965.2021.0776(in Chinese)
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Lithium-ion batteries have been used in high-altitude areas and airports in China, and therefore it is urgent to investigate their cycle performance and aging mechanism in high-altitude and low-pressure environments. The aging behavior of NCM523 pouch lithium-ion batteries is analyzed in terms of electrochemical characteristics such as battery health status, charging energy, direct current internal resistance, electrochemical impedance spectroscopy, capacity increase and differential voltage curves under 96 kPa-25℃ (normal temperature and pressure) and 60 kPa-25℃ (normal temperature and low pressure). The results show that the low pressure of 60 kPa accelerates the aging process of lithium-ion batteries. The internal structure of the battery is affected by low pressure, which increases the ohmic resistance and charge transfer resistance of the battery by 6.22% and 45.76%, respectively, compared with those under normal pressure. In addition, the lithium deintercalation reaction is limited, and the kinetic properties of the battery interface are reduced. Due to the increase of the battery impedance, the cycle capacity decays rapidly, determined by the loss of active Li+ of the cathode. The attenuation rate of the battery health state is higher by 3.08% than that under atmospheric pressure.
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